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Ronnie O'Sullivan lost 4-0 to Shaun Murphy at the Champion of Champions in Leicester.
The defeat follows O'Sullivan's earlier exit at the Northern Ireland Open against Ka Wai Cheung.
Shaun Murphy secured victory with breaks including a 68 and closed out a tense fourth frame 61-42.
Murphy will face Chang Bingyu in the quarter-finals after Chang defeated Wu Yize 4-3.
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